Sunday, July 29, 2018

NET Power, Supercritical CO2 Technology, and the Development of the First Allam Cycle Natural GAs Power Plants: Featuring Carbon Capture, No Pollution, and Comparable Efficiencies to Existing Combined-Cycle Gas Plants


NET Power, Supercritical CO2 Technology, and the Development of the First Allam Cycle Natural Gas Power Plants: Featuring Carbon, No Pollution, and Comparable Efficiencies and Costs to Existing Combined -Cycle Gas Plants

Durham, North Carolina company NET Power announced a few weeks ago that they fired up their new $140 million 50MW test plant in LaPorte, Texas that runs on natural gas and captures the CO2 at no additional cost to other modern gas plants when done at scale. This is a big deal, possibly a very big deal. It is good for natural gas. It is good for decarbonization. It is good for pollution abatement. It is good for electricity consumers. It is good for people who live nearby who otherwise might be close to a major pollution source. This is likely to be a major victory for carbon capture technology. The main limiting factor to scaling this technology is the need for sequestration and/or to sell the by-products – mainly CO2, nitrogen, and argon. Oil companies purchase CO2 for CO2 flooding to recover oil and related plastics companies use it in making ethylene. Another advantage of these types of plants is that they have a smaller physical footprint than current natural gas combined cycle plants. NET Power’s parent company 8 Rivers Capitol is funding ongoing tech development, Exelon Generation is operating the plant, and Toshiba is working on turbine development. The plants also use far less water for cooling and could even be air cooled if necessary. They think that they will surpass the economics of a conventional modern combined cycle gas plant when they scale up, with the 30th plant (presumably 300MW).



Supercritical CO2

The key to the plant’s function is supercritical CO2, which is CO2 that is heated to a certain temperature (31.1 deg C – a hot day in Phoenix) and pressurized to 7.39 megapascals. This makes the CO2 expand like a gas but flow like a liquid. Liquids can be pumped. The CO2 is compressed, pumped, and guided to spin a turbine. It is compressed to the needed pressure then pumped since pumping requires far less energy than compression. That is one key to its lower costs. It is the pressurized supercritical CO2 (SCO2) itself that runs the turbine.

Oxyfuel Combustion

Like combined-cycle gas plants the exhaust from combusting the gas in near-pure oxygen runs a turbine (here by heating CO2 to run the turbine), but instead of the second cycle being still-hot exhaust heating steam to run a second turbine the second cycle uses the waste heat to reheat the next batch of CO2 so that the heat is basically recycled. The plant also relies on oxyfuel combustion, or oxy-firing. This involves burning in pure oxygen. It was tried in the past in coal projects with limited results but works better in natural gas combustion, presumably due to less impurities in gas relative to coal. Using it for coal also requires a desulfurization system and generates waste in the form of sulfur and heavy metals. Oxyfuel combustion has been in common use for some time in other industries such as aluminum, steel, and glass. Nitrogen, which makes up over 70% of air, is removed. Another problem with coal is the ash it generates which gets sticky and is hard to handle. It is oxyfuel combustion that causes the waste stream from the combustion to be basically pure CO2, with magnitudes less impurities than a traditional combustion system. This makes carbon capture vastly easier and cheaper.

The Allam Cycle

UK engineer Rodney Allam is credited with the invention of the Allam Cycle. Allam has defined it as “a high-pressure, highly recuperative, oxyfuel, supercritical CO2 cycle.” The combustible mix by mass is 94% CO2, 4.75% oxygen, and 1.25% natural gas. The pressurized CO2 runs the fluid turbine (different from a steam turbine). Apparently, much of the CO2 can be reused (thus the term “highly recuperative”), some water is condensed out, and some 90+% pure CO2 (considered a pipeline-quality CO2 product) is ready for utilization or sequestration. It is unclear just how much CO2 is used up in the process and how much is produced as a by-product that must be utilized and/or sequestered. Allam notes that the process is not “parasitic, “or added on, as are all other conventional carbon capture technologies. He describes it this way in the 2013 Modern Power Systems article referenced below:

NET Power turns the CO2 problem into the solution by exploiting the special thermodynamic properties of carbon dioxide as a working fluid. This avoids the energy losses that steam-based cycles encounter as a result of heat loss inherent in the unavoidable vaporization and condensation of water. In the process, NET Power generates - at no additional cost - a high-pressure, high-quality CO2 byproduct that is ready for pipeline removal.

The process is termed “highly recuperative for a number of reasons: 1) much of the CO2 is recycled, 2) waste-heat from the air compressors of the cryogenic air separation plant associated with the oxy-combustion system (oxy-combustion is normally much more parasitic) is recycled to reheat the recycled CO2 – thus the heat-exchange process is highly efficient , 3) the energy savings from running compression to running pumps as the CO2 gets into a supercritical state, and 4) the CO2 is removed from the recycle flow at high purity and at pressures which can flow in a CO2 pipeline – it is both pipeline quality and pipeline ready.

Of course, the projects will be initially confined to places where the extra CO2 can be used which requires both a market for the CO2 and some CO2 pipeline infrastructure. Thus, it is likely to be confined to projects near major secondary oil recovery operations. He also notes that Toshiba is well-positioned to build the turbines required as they have the expertise in high pressure turbines, materials, and manufacture. The NET Power cycle systems are cheaper due to smaller footprint (in part due to higher pressures) and the lack of a need for smokestacks and emissions control systems. This saved cost is partially offset by NET Power’s requirements for a cryogenic air separation unit and a heat exchanger block.

Allam also mentions the NET Power cycle as a ‘platform’ that can be used for other processes such as a coal plant, LNG regasification facilities where it could increase efficiencies, hybrid concentrated solar-natural gas plants where it could increase efficiencies, by superheating steam at greater efficiencies than current in steam cycle turbines, and direct link-up to secondary recovery of oil where associated gas could be the combustible source. He also notes that the NET Power cycle can be utilized for coal just as readily and this could be useful for countries reliant on coal like India and China, although it is unclear what they could do with the excess CO2. 


Marketing CO2 and Other Gases

Finding a market for the captured CO2, nitrogen, argon, and a few other gases is a current focus. Power plants near oil fields could provide CO2 for enhanced oil recovery. The pure CO2 could even be used as a source to make gasoline or ethanol as analyses show these new processes to be economically viable at scale, especially CO2-to-ethanol. Of course, the extra CO2 could also be sequestered which would render the projects less economic and perhaps uneconomic. Perhaps they could even send some to Europe who has a current shortage of food-grade CO2 for things like carbonated beverages – although it is a temporary shortage due to plant maintenance! I wonder if CO2 in whatever state could also be utilized for energy storage – of the compressed air type. Indications are that the CO2-to-ethanol chemical reaction has very low energy input requirements and could very well be developed for energy storage, especially of intermittent renewables in times of overgeneration. Carbon capture, utilization, and sequestration (CCUS) has been at an economic standstill for some time since critics have argued that renewables, especially wind, are cheaper to deploy without CCUS than fitting fossil fuel plants with CCUS. The Vox article explores the problem of what to do with the CO2 and who pays for its sequestration. If the plant pays then the economics go way down. If the public pays then it becomes a fossil fuel subsidy. Of course, if there is a taker or buyer then the economics stay the same or get better.

The Current State of Carbon Capture, Utilization, and Sequestration (CCUS)

According to the article referenced below about the new clean energy incentives bill signed by Trump:

“Currently, there are 17 large-scale carbon capture plants in the world, sequestering 40 million metric tons of carbon dioxide in total—about 0.1% of total global emissions.”

That is a dismally small amount and critics probably correctly point out that CCUS seems unlikely to make a major impact on carbon emissions, especially in the near-term, as the costs have been consistently too high. The International Energy Agency suggests that by 2050 the global need for CCUS will be for 6 billion metric tons to be diverted from the atmosphere – or about 15% of emissions. This will be unlikely to happen without efficiency, cost, and technological improvements.  

Public perception of CCUS has waned over the years as the technology has stagnated. With wind and solar an added advantage is companies and residents that want zero or low emissions technologies. It is unclear if and probably unlikely that low-emitting tech that still uses fossil fuels will be as warmly welcomed and pursued in things like power purchase agreements. Thus, I doubt companies like Google, Amazon, or Facebook, would embrace the tech over wind and solar for their data centers, for example.

US DOE Energy Research Contributes to Technology Solutions

The National Energy Technology Laboratory (NETL) is involved with several research projects utilizing supercritical CO2 as well as turbine development, carbon capture, and sequestration. They are involved with R&D in several SCO2 cycles and turbomachinery in their Advanced Turbines Program. Their current projects include working with what’s called the Brayton Cycle which is a closed-loop system that is also non-condensing. The Alam Cycle involves condensing out water but could run without doing so at additional loss of efficiency – so added cost. The Brayton Cycle and other SCO2 cycles may work better with oxy-combusted coal. A 10MW natural gas test plant of the Brayton Cycle will open in Texas in 2019. Other SCO2 projects include ‘indirect firing’ which utilizes turbine waste heat to heat SCO2 in a conventional Combined Cycle Gas Plant steam cycle for a 2-4% increase in efficiency for little cost. Other projects involve converting waste heat from turbines and/or engines to heat SCO2 for a 20% increase in efficiency at a small scale. In the Netherlands Statoil, Mitsubishi, and other companies are working on a combined cycle gas plant that burns 30% hydrogen for a 10% reduction in emissions, although that project does not use SCO2 or oxyfuel combustion. Sequestration and utilization of CO2 also require transportation to point of use or sequestration, either via truck or pipeline so that is another area of expense and research. Obviously, being close to area of utilization and/or sequestration is an economic advantage.

There are also other incentives including a recently passed federal law that gives tax credits of $50 per metric ton of CO2 buried or $30 per metric ton of CO2 captured and used for oil production. These are the 45Q tax credits and plants beginning construction before 2024 are eligible and credits can be taken for 12 years.

References:

That Natural Gas Power Plant with No Carbon Emissions or Air Pollution? It Works: The Carbon-Capture Game is About to Change – by David Roberts, in Vox, June 1, 2018

This Natural Gas Plant Could Be A Big Breakthrough – by Nathanael Johnson, in Grist, May 31, 2018

NET Power Achieves Major Milestone for Carbon Capture with Demonstration Plant First Fire – Cision PR Newswire, May 30, 2018

This Power Plant Runs on CO2:  Carbon Capture Costs Nothing in NET Power’s New Plant, Which Uses Supercritical Carbon Dioxide to Drive a Turbine – by David Wagman, in IEEE Spectrum, May 30, 2018

Winner: Restoring Coal’s Sheen: Swedish Energy Company Takes a Novel Approach to Carbon Capture – by William Sweet, in IEEE Spectrum, Jan. 1, 2008

Supercritical CO2 Turbomachinery: Technology Development for Supercritical Carbon Dioxide (SCO2) Based Power Cycles – by National Energy Technology Laboratory (NETL) – website

NET Power’s CO2 Cycle: The Breakthrough that CCS Needs – by Rodney Allam, in Modern Power Systems (modernpowersystems.com), July 2013

Trump signed a landmark bill that could create the next big technologies to fight climate change – by Akshat Rathi, in Quartz (qtz.com), Feb 9, 2018

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